|
|
The dielectric function of PbS quantum dots in a glass matrix |
Optical Materials Express, Vol. 2, Issue 5, pp. 496-500 (2012)
http://dx.doi.org/10.1364/OME.2.000496
Enhanced HTML
Acrobat PDF (836 KB)
Abstract
The dielectric function of PbS quantum dots (Qdots) with diameters of 3.5-5.0 nm in glass matrix is determined from transmission measurements by Maxwell-Garnett effective medium theory combined with iterative Kramers-Kronig analysis. The algorithm used provides real and imaginary part of the dielectric function in the 200-1800 nm spectral range, for both Qdot-doped glasses as well as the PbS Qdots alone. The latter data are compared with the results obtained from colloidal PbS quantum dots and, within the limits of the experimental error, agreement is found.
© 2012 OSA
OCIS Codes
(120.4530) Instrumentation, measurement, and metrology : Optical constants
(300.1030) Spectroscopy : Absorption
(260.2065) Physical optics : Effective medium theory
(160.4236) Materials : Nanomaterials
ToC Category:
Nanomaterials
History
Original Manuscript: December 12, 2011
Revised Manuscript: March 12, 2012
Manuscript Accepted: March 12, 2012
Published: April 2, 2012
Virtual Issues
Quantum Dots for Photonic Applications (2012) Optical Materials Express
Citation
Iwan Moreels, Detlef Kruschke, Peter Glas, and Jens W. Tomm, "The dielectric function of PbS quantum dots in a glass matrix," Opt. Mater. Express 2, 496-500 (2012)
http://www.opticsinfobase.org/ome/abstract.cfm?URI=ome-2-5-496
Sort: Year | Journal | Reset
References
- A. Olkhovets, R. C. Hsu, A. Lipovskii, and F. W. Wise, “Size-dependent temperature variation of the energy gap in lead-salt quantum dots,” Phys. Rev. Lett.81(16), 3539–3542 (1998). [CrossRef]
- G. Konstantatos, C. J. Huang, L. Levina, Z. H. Lu, and E. H. Sargent, “Efficient infrared electroluminescent devices using solution-processed colloidal quantum dots,” Adv. Funct. Mater.15(11), 1865–1869 (2005). [CrossRef]
- K. Wundke, J. Auxier, A. Schulzgen, N. Peyghambarian, and N. F. Borrelli, “Room-temperature gain at 1.3 mu m in PbS-doped glasses,” Appl. Phys. Lett.75(20), 3060–3062 (1999). [CrossRef]
- S. A. McDonald, G. Konstantatos, S. G. Zhang, P. W. Cyr, E. J. D. Klem, L. Levina, and E. H. Sargent, “Solution-processed PbS quantum dot infrared photodetectors and photovoltaics,” Nat. Mater.4(2), 138–142 (2005). [CrossRef] [PubMed]
- S. Günes, K. P. Fritz, H. Neugebauer, N. S. Sariciftci, S. Kumar, and G. D. Scholes, “Hybrid solar cells using PbS nanoparticles,” Sol. Energy Mater. Sol. Cells91(5), 420–423 (2007). [CrossRef]
- P. T. Guerreiro, S. Ten, N. F. Borrelli, J. Butty, G. E. Jabbour, and N. Peyghambarian, “PbS quantum-dot doped grasses as saturable absorbers for mode locking of a Cr:forsterite laser,” Appl. Phys. Lett.71(12), 1595–1597 (1997). [CrossRef]
- L. Levina, W. Sukhovatkin, S. Musikhin, S. Cauchi, R. Nisman, D. P. Bazett-Jones, and E. H. Sargent, “Efficient infrared-emitting PbS quantum dots grown on DNA and stable in aqueous solution and blood plasma,” Adv. Mater. (Deerfield Beach Fla.)17(15), 1854–1857 (2005). [CrossRef]
- M. Kim and M. Yoda, “Infrared quantum dots for liquid-phase thermometry in silicon,” Meas. Sci. Technol.22(8), 085401 (2011). [CrossRef]
- I. Moreels, G. Allan, B. De Geyter, L. Wirtz, C. Delerue, and Z. Hens, “Dielectric function of colloidal lead chalcogenide quantum dots obtained by a Kramers-Kronig analysis of the absorbance spectrum,” Phys. Rev. B81(23), 235319 (2010). [CrossRef]
- N. F. Borrelli and D. W. Smith, “Quantum confinement of PbS microcrystals in glass,” J. Non-Cryst. Solids180(1), 25–31 (1994). [CrossRef]
- K. E. Fox, T. Furukawa, and W. B. White, “Transition-metal ions in silicate melts. Part 2. Iron in sodium-silicate glasses,” Phys. Chem. Glasses23, 169–178 (1982).
- I. Moreels, K. Lambert, D. Smeets, D. De Muynck, T. Nollet, J. C. Martins, F. Vanhaecke, A. Vantomme, C. Delerue, G. Allan, and Z. Hens, “Size-dependent optical properties of colloidal PbS quantum dots,” ACS Nano3(10), 3023–3030 (2009). [CrossRef] [PubMed]
- A. Sihvola, “Two main avenues leading to the Maxwell Garnett mixing rule,” J. Electromagn. Waves Appl.15(6), 715–725 (2001). [CrossRef]
Cited By |
OSA is able to provide readers links to articles that cite this paper by participating in CrossRef's Cited-By Linking service. CrossRef includes content from more than 3000 publishers and societies. In addition to listing OSA journal articles that cite this paper, citing articles from other participating publishers will also be listed.





OSA is a member of 