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Virtual Journal for Biomedical Optics

Virtual Journal for Biomedical Optics

| EXPLORING THE INTERFACE OF LIGHT AND BIOMEDICINE

  • Editor: Gregory W. Faris
  • Vol. 3, Iss. 6 — Jun. 17, 2008

Excitation and emission enhancement of single molecule fluorescence through multiple surface-plasmon resonances on metal trimer nanoantennas

V. Giannini and J. A. Sánchez-Gil  »View Author Affiliations


Optics Letters, Vol. 33, Issue 9, pp. 899-901 (2008)
http://dx.doi.org/10.1364/OL.33.000899


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Abstract

We study theoretically the light scattering from trimers of metal nanowires, with emphasis on the occurrence of multiple surface-plasmon resonances, showing that such resonances can be exploited to achieve twofold-enhanced fluorescence from a single molecule placed in the nanotrimer gaps, even if excitation and emission frequencies are separated. Pump enhancement stems from the local field enhancement coinciding with one of the resonances, whereas a strong enhancement of the radiative decay rate (and quantum yield) is revealed at a different resonance, leading to a large overall signal emission.

© 2008 Optical Society of America

OCIS Codes
(240.6680) Optics at surfaces : Surface plasmons
(260.2510) Physical optics : Fluorescence
(290.5850) Scattering : Scattering, particles
(160.4236) Materials : Nanomaterials

ToC Category:
Physical Optics

History
Original Manuscript: December 14, 2007
Revised Manuscript: February 19, 2008
Manuscript Accepted: February 24, 2008
Published: April 21, 2008

Virtual Issues
Vol. 3, Iss. 6 Virtual Journal for Biomedical Optics

Citation
V. Giannini and J. A. Sánchez-Gil, "Excitation and emission enhancement of single molecule fluorescence through multiple surface-plasmon resonances on metal trimer nanoantennas," Opt. Lett. 33, 899-901 (2008)
http://www.opticsinfobase.org/vjbo/abstract.cfm?URI=ol-33-9-899


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References

  1. U. Kreibig and M. Vollmer, Optical Properties of Metal Clusters (Springer, 1995).
  2. W. L. Barnes, A. Dereux, and T. W. Ebbesen, Nature 424, 824 (2003). [CrossRef] [PubMed]
  3. H. Xu, J. Aizpurua, M. Käll, and P. Apell, Phys. Rev. E 62, 4318 (2000). [CrossRef]
  4. J. P. Kottmann, O. J. F. Martin, D. R. Smith, and S. Schultz, Phys. Rev. B 64, 235402 (2001). [CrossRef]
  5. K. L. Kelly, E. Coronado, L. L. Zhao, and G. C. Schatz, J. Phys. Chem. B 107, 668 (2003). [CrossRef]
  6. J. Aizpurua, G. W. Bryant, L. J. Richter, F. J. García de Abajo, B. K. Kelley, and T. Mallouk, Phys. Rev. B 71, 235420 (2005). [CrossRef]
  7. P. Nordlander, C. Oubre, E. Prodan, K. Li, and M. I. Stockman, Nano Lett. 4, 899 (2004). [CrossRef]
  8. D. P. Fromm, A. Sundaramurthy, P. J. Schuck, G. Kino, and W. E. Moerner, Nano Lett. 4, 957 (2004). [CrossRef]
  9. P. J. Schuck, D. P. Fromm, A. Sundaramurthy, G. S. Kino, and W. E. Moerner, Phys. Rev. Lett. 94, 017402 (2005). [CrossRef] [PubMed]
  10. P. Mühlschlegel, H. J. Eisler, O. J. F. Martin, B. Hecht, and D. W. Pohl, Science 308, 1607 (2005). [CrossRef] [PubMed]
  11. K. L. Shuford, M. A. Ratner, and G. C. Schatz, J. Chem. Phys. 123, 114713 (2005). [CrossRef]
  12. I. Romero, J. Aizpurua, G. W. Bryant, and F. J. García de Abajo, Opt. Express 14, 9988 (2006). [CrossRef] [PubMed]
  13. S. E. Sburlan, L. A. Blanco, and M. Nieto-Vesperinas, Phys. Rev. B 73, 035403 (2006). [CrossRef]
  14. T. Søndergaard and S. I. Bozhevolnyi, Opt. Express 15, 4198 (2007). [CrossRef] [PubMed]
  15. V. Giannini, J. A. Sánchez-Gil, J. V. García-Ramos, and E. R. Méndez, Phys. Rev. B 75, 235447 (2007). [CrossRef]
  16. J. J. Greffet, Science 308, 1561 (2005). [CrossRef] [PubMed]
  17. L. Novotny, Phys. Rev. Lett. 98, 266802 (2007). [CrossRef] [PubMed]
  18. L. Rogobete, F. Kaminski, M. Agio, and V. Sandoghdar, Opt. Lett. 32, 1623 (2007). [CrossRef] [PubMed]
  19. O. Muskens, V. Giannini, J. A. Sánchez-Gil, and J. Gómez Rivas, Nano Lett. 7, 2871 (2007). [CrossRef] [PubMed]
  20. V. Giannini and J. A. Sánchez-Gil, J. Opt. Soc. Am. A 24, 2822 (2007). [CrossRef]
  21. P. B. Johnson and R. W. Christy, Phys. Rev. B 6, 4370 (1972). [CrossRef]
  22. H. Wang, D. W. Brandl, P. Nordlander, and N. J. Halas, Acc. Chem. Res. 40, 53 (2007). [CrossRef] [PubMed]
  23. R. R. Chance, A. Prock, and R. Silbey, Adv. Chem. Phys. 37, 1 (1978). [CrossRef]
  24. R. Carminati, J.-J. Greffet, C. Henkel, and J. M. Vigoureux, Opt. Commun. 261, 368 (2006). [CrossRef]
  25. P. Bharadwaj and L. Novotny, Opt. Express 15, 14266 (2007). [CrossRef] [PubMed]
  26. J. R. Lakowicz, Anal. Biochem. 337, 171 (2005). [CrossRef] [PubMed]

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