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Virtual Journal for Biomedical Optics

Virtual Journal for Biomedical Optics

| EXPLORING THE INTERFACE OF LIGHT AND BIOMEDICINE

  • Editor: Gregory W. Faris
  • Vol. 2, Iss. 1 — Jan. 19, 2007

Multilayer Enhanced Gold Film over Nanostructure Surface-Enhanced Raman Substrates

Honggang Li, Caitlin E. Baum, Jian Sun, and Brian M. Cullum

Applied Spectroscopy, Vol. 60, Issue 12, pp. 1377-1385 (2006)


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Abstract

We have developed a novel class of gold multilayer, surface-enhanced Raman scattering (SERS) substrates that are capable of enhancing SERS signals by 15.3-fold over conventional gold film over nanostructure (GFON) SERS substrates, making them comparable in sensitivity to optimized silver film over nanostructure (SFON) substrates, while providing the long-term stability obtained from gold. They are fabricated by depositing 10 Å thick silver oxide islands on conventional GFON substrates, followed by deposition of a second continuous gold layer. The silver oxide layer acts as a dielectric spacer between the two continuous gold films and produces significantly enhanced SERS signals, as compared to optimized single layer substrates of the same geometry or comparable substrates prepared by deposition of silver islands that are not oxidized. In addition to the enhanced sensitivity of these multilayer substrates, they also exhibit long SERS active shelf-lives (i.e., months), with no measurable degradation in SERS enhancement, and relative standard deviations in SERS enhancement of less than 5.2% across the substrate's surface.

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Vol. 2, Iss. 1 Virtual Journal for Biomedical Optics

Citation
Honggang Li, Caitlin E. Baum, Jian Sun, and Brian M. Cullum, "Multilayer Enhanced Gold Film over Nanostructure Surface-Enhanced Raman Substrates," Appl. Spectrosc. 60, 1377-1385 (2006)
http://www.opticsinfobase.org/vjbo/abstract.cfm?URI=as-60-12-1377

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