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Anomalous enhanced emission from PbS quantum dots on a photonic-crystal microcavityTing Shan Luk, Shisheng Xiong, Weng W. Chow, Xiaoyu Miao, Ganapathi Subramania, Paul J. Resnick, Arthur J. Fischer, and Jeffrey C. Brinker »View Author Affiliations
Ting Shan Luk,1,2,*
Shisheng Xiong,3
Weng W. Chow,2,4
Xiaoyu Miao,5
Ganapathi Subramania,2
Paul J. Resnick,2
Arthur J. Fischer,2
and Jeffrey C. Brinker2,3
1Center for Integrated NanoTechnologies, Sandia National Laboratories, Albuquerque, New Mexico 87123, USA 2Sandia National Laboratories, Albuquerque, New Mexico 87185-1086, USA 3Center for MicroEngineered Materials, Department of Chemical and Nuclear Engineering, University of New Mexico, Albuquerque, New Mexico 87106, USA 4Physics Department and Institute of Quantum Studies, Texas A&M University, College Station, Texas 77843, USA 5Google Inc., 1600 Amphitheatre Parkway, Mountain View, California 94043, USA *Corresponding author: tsluk@sandia.gov |
JOSA B, Vol. 28, Issue 6, pp. 1365-1373 (2011)
http://dx.doi.org/10.1364/JOSAB.28.001365
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Abstract
We report up to 75 times enhancement in emission from lithographically produced photonic crystals with postprocessing close-packed colloidal quantum-dot incorporation. In our analysis, we use the emission from a close-packed free-standing film as a reference. After discounting the angular redistribution effect, our analysis shows that the observed enhancement is larger than the combined effects of Purcell enhancement and dielectric enhancement with the microscopic local field. The additional enhancement mechanisms, which are consistent with all our observations, are thought to be spectral diffusion mediated by phonons and local polarization fluctuations that allow off-resonant excitons to emit at the cavity wavelengths.
© 2011 Optical Society of America
OCIS Codes
(230.0230) Optical devices : Optical devices
(300.2140) Spectroscopy : Emission
(140.3945) Lasers and laser optics : Microcavities
(350.4238) Other areas of optics : Nanophotonics and photonic crystals
ToC Category:
Lasers and Laser Optics
History
Original Manuscript: February 15, 2011
Manuscript Accepted: March 23, 2011
Published: May 9, 2011
Virtual Issues
Vol. 6, Iss. 7 Virtual Journal for Biomedical Optics
Citation
Ting Shan Luk, Shisheng Xiong, Weng W. Chow, Xiaoyu Miao, Ganapathi Subramania, Paul J. Resnick, Arthur J. Fischer, and Jeffrey C. Brinker, "Anomalous enhanced emission from PbS quantum dots on a photonic-crystal microcavity," J. Opt. Soc. Am. B 28, 1365-1373 (2011)
http://www.opticsinfobase.org/vjbo/abstract.cfm?URI=josab-28-6-1365
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