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Role of in-plane polarizability of the tip in scattering near-field microscopy of a plasmonic nanoparticleDeok-Soo Kim and Zee Hwan Kim »View Author Affiliations
Deok-Soo Kim
and Zee Hwan Kim*
Department of Chemistry, Korea University, Anam-Dong, Seongbuk-Gu, Seoul 136-701, Korea *Corresponding author: zhkim@korea.ac.kr |
Optics Express, Vol. 20, Issue 8, pp. 8689-8699 (2012)
http://dx.doi.org/10.1364/OE.20.008689
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Abstract
We report that a pyramid-shaped scanning probe microscopy tip has non-zero polarizability along the in-plane direction (perpendicular to the tip axis, z) at visible frequency. The in-plane polarizability enables the scattering-type scanning near-field optical microscopy (s-SNOM) to measure the in-plane field component around a plasmon-resonant nanoparticle. Because of the non-zero in-plane polarizability, the cross-polarized s-SNOM images may contain contributions from the in-plane field component of an out-of-plane plasmon mode as well as the out-of-plane field component of an in-plane mode. By comparing a scattering model and experimental s-SNOM images, we estimate the polarization anisotropies of pyramid-shaped Si-tips and metal-coated Si-tips.
© 2012 OSA
OCIS Codes
(240.6680) Optics at surfaces : Surface plasmons
(180.4243) Microscopy : Near-field microscopy
ToC Category:
Microscopy
History
Original Manuscript: February 8, 2012
Revised Manuscript: March 22, 2012
Manuscript Accepted: March 24, 2012
Published: March 29, 2012
Virtual Issues
Vol. 7, Iss. 6 Virtual Journal for Biomedical Optics
Citation
Deok-Soo Kim and Zee Hwan Kim, "Role of in-plane polarizability of the tip in scattering near-field microscopy of a plasmonic nanoparticle," Opt. Express 20, 8689-8699 (2012)
http://www.opticsinfobase.org/vjbo/abstract.cfm?URI=oe-20-8-8689
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References
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- R. Esteban, R. Vogelgesang, J. Dorfmüller, A. Dmitriev, C. Rockstuhl, C. Etrich, and K. Kern, “Direct near-field optical imaging of higher order plasmonic resonances,” Nano Lett.8(10), 3155–3159 (2008). [CrossRef] [PubMed]
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- M. Schnell, A. Garcia-Etxarri, J. Alkorta, J. Aizpurua, and R. Hillenbrand, “Phase-resolved mapping of the near-field vector and polarization state in nanoscale antenna gaps,” Nano Lett.10(9), 3524–3528 (2010). [CrossRef] [PubMed]
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- B. S. Guiton, V. Iberi, S. Li, D. N. Leonard, C. M. Parish, P. G. Kotula, M. Varela, G. C. Schatz, S. J. Pennycook, and J. P. Camden, “Correlated optical measurements and plasmon mapping of silver nanorods,” Nano Lett.11(8), 3482–3488 (2011). [CrossRef] [PubMed]
- H. Wei, Z. Li, X. Tian, Z. Wang, F. Cong, N. Liu, S. Zhang, P. Nordlander, N. J. Halas, and H. Xu, “Quantum dot-based local field imaging reveals plasmon-based interferometric logic in silver nanowire networks,” Nano Lett.11(2), 471–475 (2011). [CrossRef] [PubMed]
- D.-S. Kim, J. Heo, S.-H. Ahn, S. W. Han, W. S. Yun, and Z. H. Kim, “Real-space mapping of the strongly coupled plasmons of nanoparticle dimers,” Nano Lett.9(10), 3619–3625 (2009). [CrossRef] [PubMed]
- A. McLeod, A. Weber-Bargioni, Z. Zhang, S. Dhuey, B. Harteneck, J. B. Neaton, S. Cabrini, and P. J. Schuck, “Nonperturbative visualization of nanoscale plasmonic field distributions via photon localization microscopy,” Phys. Rev. Lett.106(3), 037402 (2011). [CrossRef] [PubMed]
- J. Nelayah, M. Kociak, O. Stephan, F. J. G. de Abajo, M. Tence, L. Henrard, D. Taverna, I. Pastoriza-Santos, L. M. Liz-Marzan, and C. Colliex, “Mapping surface plasmons on a single matallic nanoparticle,” Nat. Phys.3(5), 348–353 (2007). [CrossRef]
- D.-S. Kim, J. Heo, S.-H. Ahn, S. W. Han, W. S. Yun, and Z. H. Kim, “Real-space mapping of the strongly coupled plasmons of nanoparticle dimers,” Nano Lett.9(10), 3619–3625 (2009). [CrossRef] [PubMed]
- P. Alonso-González, P. Albella, M. Schnell, J. Chen, F. Huth, A. García-Etxarri, F. Casanova, F. Golmar, L. Arzubiaga, L. E. Hueso, J. Aizpurua, and R. Hillenbrand, “Resolving the electromagnetic mechanism of surface-enhanced light scattering at single hot spots,” Nat. Commun3, 684 (2012). [CrossRef] [PubMed]
- M. Schnell, P. Alonso-Gonzalez, L. Arzubiaga, F. Casanova, L. E. Hueso, A. Chuvilin, and R. Hillenbrand, “Nanofocusing of mid-infrared energy with tapered transmission lines,” Nat. Photonics5(5), 283–287 (2011). [CrossRef]
- M. Schnell, A. Garcia-Etxarri, J. Alkorta, J. Aizpurua, and R. Hillenbrand, “Phase-resolved mapping of the near-field vector and polarization state in nanoscale antenna gaps,” Nano Lett.10(9), 3524–3528 (2010). [CrossRef] [PubMed]
- M. Schnell, A. Garcia-Etxarri, A. J. Huber, K. B. Crozier, A. Borisov, J. Aizpurua, and R. Hillenbrand, “Amplitude- and phase-resolved near-field mapping of infrared antenna modes by transmission-mode scattering-type near-Field microscopy,” J. Phys. Chem. C114(16), 7341–7345 (2010). [CrossRef]
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- J. Dorfmüller, R. Vogelgesang, R. T. Weitz, C. Rockstuhl, C. Etrich, T. Pertsch, F. Lederer, and K. Kern, “Fabry-Pérot resonances in one-dimensional plasmonic nanostructures,” Nano Lett.9(6), 2372–2377 (2009). [CrossRef] [PubMed]
- K. G. Lee, H. W. Kihm, J. E. Kihm, W. J. Choi, H. Kim, C. Ropers, D. J. Park, Y. C. Yoon, S. B. Choi, D. H. Woo, J. Kim, B. Lee, Q. H. Park, C. Lienau, and D. S. Kim, “Vector field microscopic imaging of light,” Nat. Photonics1(1), 53–56 (2007). [CrossRef]
- H. Wei, Z. Li, X. Tian, Z. Wang, F. Cong, N. Liu, S. Zhang, P. Nordlander, N. J. Halas, and H. Xu, “Quantum dot-based local field imaging reveals plasmon-based interferometric logic in silver nanowire networks,” Nano Lett.11(2), 471–475 (2011). [CrossRef] [PubMed]
- K. G. Lee, H. W. Kihm, J. E. Kihm, W. J. Choi, H. Kim, C. Ropers, D. J. Park, Y. C. Yoon, S. B. Choi, D. H. Woo, J. Kim, B. Lee, Q. H. Park, C. Lienau, and D. S. Kim, “Vector field microscopic imaging of light,” Nat. Photonics1(1), 53–56 (2007). [CrossRef]
- D.-S. Kim, J. Heo, S.-H. Ahn, S. W. Han, W. S. Yun, and Z. H. Kim, “Real-space mapping of the strongly coupled plasmons of nanoparticle dimers,” Nano Lett.9(10), 3619–3625 (2009). [CrossRef] [PubMed]
- H. Wei, Z. Li, X. Tian, Z. Wang, F. Cong, N. Liu, S. Zhang, P. Nordlander, N. J. Halas, and H. Xu, “Quantum dot-based local field imaging reveals plasmon-based interferometric logic in silver nanowire networks,” Nano Lett.11(2), 471–475 (2011). [CrossRef] [PubMed]
- A. McLeod, A. Weber-Bargioni, Z. Zhang, S. Dhuey, B. Harteneck, J. B. Neaton, S. Cabrini, and P. J. Schuck, “Nonperturbative visualization of nanoscale plasmonic field distributions via photon localization microscopy,” Phys. Rev. Lett.106(3), 037402 (2011). [CrossRef] [PubMed]
Analyst (Lond.)
- R. Vogelgesang and A. Dmitriev, “Real-space imaging of nanoplasmonic resonances,” Analyst (Lond.)135(6), 1175–1181 (2010). [CrossRef] [PubMed]
Appl. Phys. B
- R. Hillenbrand and F. Keilmann, “Optical oscillation modes of plasmon particles observed in direct space by phase-contrast near-field microscopy,” Appl. Phys. B73(3), 239–243 (2001). [CrossRef]
Chem. Phys. Lett.
- Y. Abate, A. Schwartzberg, D. Strasser, and S. R. Leone, “Nanometer-scale size dependent imaging of cetyl trimethyl ammonium bromide (CTAB) capped and uncapped gold nanoparticles by apertureless near-field optical microscopy,” Chem. Phys. Lett.474(1–3), 146–152 (2009). [CrossRef]
J. Appl. Phys.
- J. Sun, P. S. Carney, and J. C. Schotland, “Strong tip effects in near-field scanning optical tomography,” J. Appl. Phys.102(10), 103103 (2007). [CrossRef]
J. Phys. Chem. C
- M. Schnell, A. Garcia-Etxarri, A. J. Huber, K. B. Crozier, A. Borisov, J. Aizpurua, and R. Hillenbrand, “Amplitude- and phase-resolved near-field mapping of infrared antenna modes by transmission-mode scattering-type near-Field microscopy,” J. Phys. Chem. C114(16), 7341–7345 (2010). [CrossRef]
Nano Lett.
- J. Dorfmüller, R. Vogelgesang, R. T. Weitz, C. Rockstuhl, C. Etrich, T. Pertsch, F. Lederer, and K. Kern, “Fabry-Pérot resonances in one-dimensional plasmonic nanostructures,” Nano Lett.9(6), 2372–2377 (2009). [CrossRef] [PubMed]
- M. Schnell, A. Garcia-Etxarri, J. Alkorta, J. Aizpurua, and R. Hillenbrand, “Phase-resolved mapping of the near-field vector and polarization state in nanoscale antenna gaps,” Nano Lett.10(9), 3524–3528 (2010). [CrossRef] [PubMed]
- D.-S. Kim, J. Heo, S.-H. Ahn, S. W. Han, W. S. Yun, and Z. H. Kim, “Real-space mapping of the strongly coupled plasmons of nanoparticle dimers,” Nano Lett.9(10), 3619–3625 (2009). [CrossRef] [PubMed]
- H. Wei, Z. Li, X. Tian, Z. Wang, F. Cong, N. Liu, S. Zhang, P. Nordlander, N. J. Halas, and H. Xu, “Quantum dot-based local field imaging reveals plasmon-based interferometric logic in silver nanowire networks,” Nano Lett.11(2), 471–475 (2011). [CrossRef] [PubMed]
- R. Esteban, R. Vogelgesang, J. Dorfmüller, A. Dmitriev, C. Rockstuhl, C. Etrich, and K. Kern, “Direct near-field optical imaging of higher order plasmonic resonances,” Nano Lett.8(10), 3155–3159 (2008). [CrossRef] [PubMed]
- B. Deutsch, R. Hillenbrand, and L. Novotny, “Visualizing the optical interaction tensor of a gold nanoparticle pair,” Nano Lett.10(2), 652–656 (2010). [CrossRef] [PubMed]
- E. J. R. Vesseur, R. de Waele, M. Kuttge, and A. Polman, “Direct observation of plasmonic modes in au nanowires using high-resolution cathodoluminescence spectroscopy,” Nano Lett.7(9), 2843–2846 (2007). [CrossRef] [PubMed]
- Z. H. Kim, S. H. Ahn, B. Liu, and S. R. Leone, “Nanometer-scale dielectric imaging of semiconductor nanoparticles: size-dependent dipolar coupling and contrast reversal,” Nano Lett.7(8), 2258–2262 (2007). [CrossRef] [PubMed]
- B. S. Guiton, V. Iberi, S. Li, D. N. Leonard, C. M. Parish, P. G. Kotula, M. Varela, G. C. Schatz, S. J. Pennycook, and J. P. Camden, “Correlated optical measurements and plasmon mapping of silver nanorods,” Nano Lett.11(8), 3482–3488 (2011). [CrossRef] [PubMed]
Nat. Commun
- P. Alonso-González, P. Albella, M. Schnell, J. Chen, F. Huth, A. García-Etxarri, F. Casanova, F. Golmar, L. Arzubiaga, L. E. Hueso, J. Aizpurua, and R. Hillenbrand, “Resolving the electromagnetic mechanism of surface-enhanced light scattering at single hot spots,” Nat. Commun3, 684 (2012). [CrossRef] [PubMed]
Nat. Photonics
- K. G. Lee, H. W. Kihm, J. E. Kihm, W. J. Choi, H. Kim, C. Ropers, D. J. Park, Y. C. Yoon, S. B. Choi, D. H. Woo, J. Kim, B. Lee, Q. H. Park, C. Lienau, and D. S. Kim, “Vector field microscopic imaging of light,” Nat. Photonics1(1), 53–56 (2007). [CrossRef]
- M. Schnell, P. Alonso-Gonzalez, L. Arzubiaga, F. Casanova, L. E. Hueso, A. Chuvilin, and R. Hillenbrand, “Nanofocusing of mid-infrared energy with tapered transmission lines,” Nat. Photonics5(5), 283–287 (2011). [CrossRef]
- M. Schnell, A. García-Etxarri, A. J. Huber, K. Crozier, J. Aizpurua, and R. Hillenbrand, “Controlling the near-field oscillations of loaded plasmonic nanoantennas,” Nat. Photonics3(5), 287–291 (2009). [CrossRef]
Nat. Phys.
- J. Nelayah, M. Kociak, O. Stephan, F. J. G. de Abajo, M. Tence, L. Henrard, D. Taverna, I. Pastoriza-Santos, L. M. Liz-Marzan, and C. Colliex, “Mapping surface plasmons on a single matallic nanoparticle,” Nat. Phys.3(5), 348–353 (2007). [CrossRef]
Opt. Express
- Z. H. Kim and S. R. Leone, “Polarization-selective mapping of near-field intensity and phase around gold nanoparticles using apertureless near-field microscopy,” Opt. Express16(3), 1733–1741 (2008). [CrossRef] [PubMed]
Phys. Rev. B
- A. Garcia-Etxarri, I. Romero, F. J. G. deAbajo, R. Hillenbrand, and J. Aizpurua, “Influence of the tip in near-field imaging of nanoparticle plasmonic modes: weak and strong coupling regimes,” Phys. Rev. B79(12), 125439 (2009). [CrossRef]
Phys. Rev. Lett.
- A. McLeod, A. Weber-Bargioni, Z. Zhang, S. Dhuey, B. Harteneck, J. B. Neaton, S. Cabrini, and P. J. Schuck, “Nonperturbative visualization of nanoscale plasmonic field distributions via photon localization microscopy,” Phys. Rev. Lett.106(3), 037402 (2011). [CrossRef] [PubMed]
- R. L. Olmon, M. Rang, P. M. Krenz, B. A. Lail, L. V. Saraf, G. D. Boreman, and M. B. Raschke, “Determination of electric-field, magnetic-field, and electric-current distributions of infrared optical antennas: a near-field optical vector network analyzer,” Phys. Rev. Lett.105(16), 167403 (2010). [CrossRef] [PubMed]
Rep. Prog. Phys.
- R. J. Potton, “Reciprocity in optics,” Rep. Prog. Phys.67(5), 717–754 (2004). [CrossRef]
Science
- T. Taubner, D. Korobkin, Y. Urzhumov, G. Shvets, and R. Hillenbrand, “Near-field microscopy through a SiC superlens,” Science313(5793), 1595 (2006). [CrossRef] [PubMed]
Other
- P. S. Carney, Personal communication, 2012.
2012, Alonso-González, Nat. Commun
- P. Alonso-González, P. Albella, M. Schnell, J. Chen, F. Huth, A. García-Etxarri, F. Casanova, F. Golmar, L. Arzubiaga, L. E. Hueso, J. Aizpurua, and R. Hillenbrand, “Resolving the electromagnetic mechanism of surface-enhanced light scattering at single hot spots,” Nat. Commun3, 684 (2012). [CrossRef] [PubMed]
- M. Schnell, P. Alonso-Gonzalez, L. Arzubiaga, F. Casanova, L. E. Hueso, A. Chuvilin, and R. Hillenbrand, “Nanofocusing of mid-infrared energy with tapered transmission lines,” Nat. Photonics5(5), 283–287 (2011). [CrossRef]
- H. Wei, Z. Li, X. Tian, Z. Wang, F. Cong, N. Liu, S. Zhang, P. Nordlander, N. J. Halas, and H. Xu, “Quantum dot-based local field imaging reveals plasmon-based interferometric logic in silver nanowire networks,” Nano Lett.11(2), 471–475 (2011). [CrossRef] [PubMed]
- A. McLeod, A. Weber-Bargioni, Z. Zhang, S. Dhuey, B. Harteneck, J. B. Neaton, S. Cabrini, and P. J. Schuck, “Nonperturbative visualization of nanoscale plasmonic field distributions via photon localization microscopy,” Phys. Rev. Lett.106(3), 037402 (2011). [CrossRef] [PubMed]
- B. S. Guiton, V. Iberi, S. Li, D. N. Leonard, C. M. Parish, P. G. Kotula, M. Varela, G. C. Schatz, S. J. Pennycook, and J. P. Camden, “Correlated optical measurements and plasmon mapping of silver nanorods,” Nano Lett.11(8), 3482–3488 (2011). [CrossRef] [PubMed]
- R. L. Olmon, M. Rang, P. M. Krenz, B. A. Lail, L. V. Saraf, G. D. Boreman, and M. B. Raschke, “Determination of electric-field, magnetic-field, and electric-current distributions of infrared optical antennas: a near-field optical vector network analyzer,” Phys. Rev. Lett.105(16), 167403 (2010). [CrossRef] [PubMed]
- M. Schnell, A. Garcia-Etxarri, A. J. Huber, K. B. Crozier, A. Borisov, J. Aizpurua, and R. Hillenbrand, “Amplitude- and phase-resolved near-field mapping of infrared antenna modes by transmission-mode scattering-type near-Field microscopy,” J. Phys. Chem. C114(16), 7341–7345 (2010). [CrossRef]
- M. Schnell, A. Garcia-Etxarri, J. Alkorta, J. Aizpurua, and R. Hillenbrand, “Phase-resolved mapping of the near-field vector and polarization state in nanoscale antenna gaps,” Nano Lett.10(9), 3524–3528 (2010). [CrossRef] [PubMed]
- B. Deutsch, R. Hillenbrand, and L. Novotny, “Visualizing the optical interaction tensor of a gold nanoparticle pair,” Nano Lett.10(2), 652–656 (2010). [CrossRef] [PubMed]
- R. Vogelgesang and A. Dmitriev, “Real-space imaging of nanoplasmonic resonances,” Analyst (Lond.)135(6), 1175–1181 (2010). [CrossRef] [PubMed]
- M. Schnell, A. García-Etxarri, A. J. Huber, K. Crozier, J. Aizpurua, and R. Hillenbrand, “Controlling the near-field oscillations of loaded plasmonic nanoantennas,” Nat. Photonics3(5), 287–291 (2009). [CrossRef]
- J. Dorfmüller, R. Vogelgesang, R. T. Weitz, C. Rockstuhl, C. Etrich, T. Pertsch, F. Lederer, and K. Kern, “Fabry-Pérot resonances in one-dimensional plasmonic nanostructures,” Nano Lett.9(6), 2372–2377 (2009). [CrossRef] [PubMed]
- D.-S. Kim, J. Heo, S.-H. Ahn, S. W. Han, W. S. Yun, and Z. H. Kim, “Real-space mapping of the strongly coupled plasmons of nanoparticle dimers,” Nano Lett.9(10), 3619–3625 (2009). [CrossRef] [PubMed]
- Y. Abate, A. Schwartzberg, D. Strasser, and S. R. Leone, “Nanometer-scale size dependent imaging of cetyl trimethyl ammonium bromide (CTAB) capped and uncapped gold nanoparticles by apertureless near-field optical microscopy,” Chem. Phys. Lett.474(1–3), 146–152 (2009). [CrossRef]
- A. Garcia-Etxarri, I. Romero, F. J. G. deAbajo, R. Hillenbrand, and J. Aizpurua, “Influence of the tip in near-field imaging of nanoparticle plasmonic modes: weak and strong coupling regimes,” Phys. Rev. B79(12), 125439 (2009). [CrossRef]
- R. Esteban, R. Vogelgesang, J. Dorfmüller, A. Dmitriev, C. Rockstuhl, C. Etrich, and K. Kern, “Direct near-field optical imaging of higher order plasmonic resonances,” Nano Lett.8(10), 3155–3159 (2008). [CrossRef] [PubMed]
- J. Sun, P. S. Carney, and J. C. Schotland, “Strong tip effects in near-field scanning optical tomography,” J. Appl. Phys.102(10), 103103 (2007). [CrossRef]
- K. G. Lee, H. W. Kihm, J. E. Kihm, W. J. Choi, H. Kim, C. Ropers, D. J. Park, Y. C. Yoon, S. B. Choi, D. H. Woo, J. Kim, B. Lee, Q. H. Park, C. Lienau, and D. S. Kim, “Vector field microscopic imaging of light,” Nat. Photonics1(1), 53–56 (2007). [CrossRef]
- J. Nelayah, M. Kociak, O. Stephan, F. J. G. de Abajo, M. Tence, L. Henrard, D. Taverna, I. Pastoriza-Santos, L. M. Liz-Marzan, and C. Colliex, “Mapping surface plasmons on a single matallic nanoparticle,” Nat. Phys.3(5), 348–353 (2007). [CrossRef]
- E. J. R. Vesseur, R. de Waele, M. Kuttge, and A. Polman, “Direct observation of plasmonic modes in au nanowires using high-resolution cathodoluminescence spectroscopy,” Nano Lett.7(9), 2843–2846 (2007). [CrossRef] [PubMed]
- Z. H. Kim, S. H. Ahn, B. Liu, and S. R. Leone, “Nanometer-scale dielectric imaging of semiconductor nanoparticles: size-dependent dipolar coupling and contrast reversal,” Nano Lett.7(8), 2258–2262 (2007). [CrossRef] [PubMed]
- T. Taubner, D. Korobkin, Y. Urzhumov, G. Shvets, and R. Hillenbrand, “Near-field microscopy through a SiC superlens,” Science313(5793), 1595 (2006). [CrossRef] [PubMed]
- R. J. Potton, “Reciprocity in optics,” Rep. Prog. Phys.67(5), 717–754 (2004). [CrossRef]
- R. Hillenbrand and F. Keilmann, “Optical oscillation modes of plasmon particles observed in direct space by phase-contrast near-field microscopy,” Appl. Phys. B73(3), 239–243 (2001). [CrossRef]
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